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Superconducting materials take the 100 K barrier

The problem of superconductivity at high temperatures is one of the central places in modern physics. So, in any case, the Nobel laureate, Academician of the Russian Academy of Sciences V. L. Ginzburg, when he gave a Nobel lecture, appealing to young physicists with a call to create a theory of superconductivity at room temperature. Interest in superconductivity is shown not only by scientists engaged in fundamental research, but also by engineers – Philips and Kavli have recently created a superconducting transistor, and Hypres has even mastered superconducting technologies as applied to cellular communications. But still, the problem of creating materials that would exhibit superconducting properties at room temperature is still not solved, and most importantly, there is no clear understanding of the essence of the phenomenon. n. high-temperature (at the boiling point of liquid nitrogen ~ 77 K) superconductivity, for example, in cuprates (copper compounds).

Photo: STM photo of doped cuprate. Impurity oxygen atoms are marked in white

A team of scientists from Cornell University in the course of research on the effect of alloying additions on superconducting properties revealed that doping of cuprates, which are dielectrics, can both lead to high-temperature superconductivity and make it impossible for the manifestation of any superconducting properties.

Atoms of dopants play the role of donors of charge carriers – electrons or “holes”, for example, bismuth-strontium-calcium-copper oxide (Bi2Sr2CaCu2O8 + x) or Bi-2212, which is an insulator, exhibits superconducting properties when an additional oxygen atom is added, which plays the role of a source “Holes”. Further doping affects the critical temperature (at which superconductivity manifests itself – zero resistance to direct current). In the theory of low-temperature superconductivity, it is shown that the phenomenon of superconductivity is due to the formation of Cooper pairs from two electrons with opposite spin in such a way that the resulting spin of the pair turns out to be zero and such a carrier becomes capable of propagating without interacting with the crystal lattice (if the electric current is constant), as expressed in zero resistance.

If at low temperatures (about 4 K) superconductivity is explained by the presence of Cooper pairs, then with high-temperature superconductivity far from everything is clear – the formation of stable Cooper pairs at high temperatures is impossible, although at one time it was suggested that such pairs are still formed , but their number constantly fluctuates, and the lifetime is small.

The latest study by scientists from Cornell University shows that doping with Bi-2212 leads to electronic disorder, and with the use of a scanning tunneling microscope (STM) it was possible to discern individual impurity atoms around which the electron density differs from what could be would expect in pure cuprate. This observation confirmed a theoretical calculation by Peter Hirschfield and colleagues from the University of Florida, who predicted that the presence of dopants distorts the local atomic and electronic structure. This leads to a noticeable change in the local pair interaction, which determines the amount of kinetic energy (depending on temperature) at which the Cooper pair is destroyed.

If the calculation is correct, then by controlling the position of the impurity atoms, it is possible to reach a higher critical temperature, which was shown by Hiroshi Eisaki and Shin-ichi Uchida, who by minimizing the “electronic disordering” caused by the presence of an impurity, managed to bring the critical temperature of Bi-2212 to almost 100 Kelvin.